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Let's say Google Scholar has a million matches for a certain keyword, but I only want to see the 100 most-cited ones. Is there any way to do this? (Note that "Sort by Relevance" doesn't accomplish this)

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    Pretty sure Web of Science lets you sort by citations.
    – Allure
    Commented Dec 8, 2023 at 22:32

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Not in Google Scholar. PubMed does not either. Both Scopus and WoS allow you to do that though. I'm not sure about other search engines or databases.

There was a similar question a few years ago: Is there an online engine like Google Scholar which allows me to sort the papers by citation count?. I'm not sure how up-to-date it still is but Dimensions and ScienceOpen should still do what you need.

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